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The university is the major seat of the Congregation of Holy Cross (albeit not its official headquarters, which are in Rome). Its main seminary, Moreau Seminary, is located on the campus across St. Joseph lake from the Main Building. Old College, the oldest building on campus and located near the shore of St. Mary lake, houses undergraduate seminarians. Retired priests and brothers reside in Fatima House (a former retreat center), Holy Cross House, as well as Columba Hall near the Grotto. The university through the Moreau Seminary has ties to theologian Frederick Buechner. While not Catholic, Buechner has praised writers from Notre Dame and Moreau Seminary created a Buechner Prize for Preaching.

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University of Notre Dame